High-resolution remote thermometry and thermography using luminescent low-dimensional tin-halide perovskites
| dc.contributor.author | Yakunin, S. | |
| dc.contributor.author | Benin, B. M. | |
| dc.contributor.author | Shynkarenko, Y. | |
| dc.contributor.author | Nazarenko, O. | |
| dc.contributor.author | Bodnarchuk, M. I. | |
| dc.contributor.author | Dirin, D. N. | |
| dc.contributor.author | et al. | |
| dc.date.accessioned | 2021-12-09T14:03:59Z | |
| dc.date.available | 2021-12-09T14:03:59Z | |
| dc.date.issued | 2019 | |
| dc.description.abstract | Although metal-halide perovskites have recently revolutionized research in optoelectronics through a unique combination of performance and synthetic simplicity, their low-dimensional counterparts can further expand the field with hitherto unknown and practically useful optical functionalities. In this context, we present the strong temperature dependence of the photoluminescence lifetime of low-dimensional, perovskite-like tin-halides and apply this property to thermal imaging. The photoluminescence lifetimes are governed by the heat-assisted de-trapping of self-trapped excitons, and their values can be varied over several orders of magnitude by adjusting the temperature (up to 20 ns degrees C-1). Typically, this sensitive range spans up to 100 degrees C, and it is both compound-specific and shown to be compositionally and structurally tunable from -100 to 110 degrees C going from [C(NH2)(3)](2)SnBr4 to Cs4SnBr6 and (C4N2H14I)(4)SnI6. Finally, through the implementation of cost-effective hardware for fluorescence lifetime imaging, based on time-of-flight technology, these thermoluminophores have been used to record thermographic videos with high spatial and thermal resolution. | |
| dc.identifier.citation | Nature Materials, vol. 18 (8), pp. 846-and, Aug 2019. | |
| dc.identifier.doi | https://doi.org/10.1038/s41563-019-0416-2 | |
| dc.identifier.uri | https://hdl.handle.net/20.500.12839/351 | |
| dc.subject | fluorescence lifetime, infrared thermography, solar-cells, efficient, time, phosphors, photons, pb, Chemistry, Materials Science, Physics | |
| dc.title | High-resolution remote thermometry and thermography using luminescent low-dimensional tin-halide perovskites | |
| dc.type | Journal Article | |
| dc.type.csemdivisions | BU-R | |
| dc.type.csemresearchareas | Other |